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Influence of metal oxide nanoparticles as antimicrobial additives embedded in waterborne coating binders based on self-crosslinking acrylic latex

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dc.title Influence of metal oxide nanoparticles as antimicrobial additives embedded in waterborne coating binders based on self-crosslinking acrylic latex en
dc.contributor.author Steinerová, Denisa
dc.contributor.author Kalendová, Andréa
dc.contributor.author Machotová, Jana
dc.contributor.author Knotek, Petr
dc.contributor.author Humpolíček, Petr
dc.contributor.author Vajďák, Jan
dc.contributor.author Šlang, Stanislav
dc.contributor.author Krejčová, Anna
dc.contributor.author Beneš, Ludvík
dc.contributor.author Wolff-Fabris, Felipe
dc.relation.ispartof Coatings
dc.identifier.issn 2079-6412 Scopus Sources, Sherpa/RoMEO, JCR
dc.date.issued 2022
utb.relation.volume 12
utb.relation.issue 10
dc.type article
dc.language.iso en
dc.publisher MDPI
dc.identifier.doi 10.3390/coatings12101445
dc.relation.uri https://www.mdpi.com/2079-6412/12/10/1445
dc.relation.uri https://www.mdpi.com/2079-6412/12/10/1445/pdf?version=1665734981
dc.subject keto-hydrazide crosslinking en
dc.subject ionic crosslinking en
dc.subject nanostructured magnesium oxide en
dc.subject zinc oxide and lanthanum oxide en
dc.subject antimicrobial activity en
dc.description.abstract This article deals with the simple preparation of environmentally friendly acrylic latex binders, which are functionalized with nanoparticles of metal oxides, namely MgO, ZnO, La2O3 and combinations of MgO and ZnO, serving as functional components to achieve antimicrobial properties, but also to improve physical-mechanical properties and chemical resilience. The incorporation of uncoated powder nanoparticles was performed during the synthesis, using the two-stage semi-continuous emulsion radical polymerization technique, to obtain latexes containing 0.5%-1.3% nanoparticles relative to the polymer content. Changes in latex performance due to nanoparticles were compared from the point of view of the type and concentration of metal oxide nanoparticles in latex. The results of the tests showed that all types of nanoparticles showed very promising properties, while with increasing concentration of nanoparticles there was an improvement in properties. The nanoparticles in latex provided interfacially crosslinked transparent smooth coating films with high gloss and good physical-mechanical properties. Latexes containing the highest concentration of nanoparticles provided coatings with significant antimicrobial activity against all tested bacterial and fungal strains, but also in-can preservative stability of liquid latex. Furthermore, the coatings were resistant to solvents, and in addition, latexes with MgO nanoparticles showed a significant decrease in the minimum film-forming temperature, and latex with a concentration of about 1.3% MgO did not show any flash corrosion under the coating film cast on a steel substrate. The latexes containing MgO and La2O3 nanoparticles provided coatings that were very resistant to water bleaching. en
utb.faculty University Institute
dc.identifier.uri http://hdl.handle.net/10563/1011206
utb.identifier.obdid 43884256
utb.identifier.scopus 2-s2.0-85140906823
utb.identifier.wok 000872490800001
utb.source j-scopus
dc.date.accessioned 2022-11-29T07:49:19Z
dc.date.available 2022-11-29T07:49:19Z
dc.description.sponsorship RP/CPS/2022/001; Ministerstvo Školství, Mládeže a Tělovýchovy, MŠMT: LM2018103
dc.description.sponsorship Ministry of Education, Youth and Sports of the Czech Republic [LM2018103]; Ministry of Education, Youth and Sports of the Czech Republic-DKRVO [RP/CPS/2022/001]
dc.rights Attribution 4.0 International
dc.rights.uri https://creativecommons.org/licenses/by/4.0/
dc.rights.access openAccess
utb.ou Centre of Polymer Systems
utb.contributor.internalauthor Humpolíček, Petr
utb.contributor.internalauthor Vajďák, Jan
utb.fulltext.affiliation Denisa Steinerová 1,* , Andréa Kalendová 1, Jana Machotová 1, Petr Knotek 2, Petr Humpolíček 3, Jan Vajdák 3, Stanislav Slang 4, Anna Krejčová 5, Ludvík Beneš 6 and Felipe Wolff-Fabris 7 1 Institute of Chemistry and Technology of Macromolecular Materials, Faculty of Chemical Technology, University of Pardubice, 532 10 Pardubice, Czech Republic 2 Department of General and Inorganic Chemistry, Faculty of Chemical Technology, University of Pardubice, 532 10 Pardubice, Czech Republic 3 Centre of Polymer Systems, Tomas Bata University in Zlín, 760 01 Zlín, Czech Republic 4 Center of Materials and Nanotechnologies, Faculty of Chemical Technology, University of Pardubice, 532 10 Pardubice, Czech Republic 5 Institute of Environmental and Chemical Engineering, Faculty of Chemical Technology, University of Pardubice, 532 10 Pardubice, Czech Republic 6 Joint Laboratory of Solid State Chemistry, Faculty of Chemical Technology, University of Pardubice, 532 10 Pardubice, Czech Republic 7 European Center for Dispersion Technologies, 95100 Selb, Germany * Correspondence: steinerovadenisa@gmail.com; Tel.: +420-727-843-211
utb.fulltext.dates Received: 19 August 2022 Revised: 25 September 2022 Accepted: 26 September 2022 Published: 30 September 2022
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utb.fulltext.sponsorship This research was funded by the Ministry of Education, Youth and Sports of the Czech Republic (project LM2018103). Authors PH and JV express thanks for project support from the Ministry of Education, Youth and Sports of the Czech Republic—DKRVO (RP/CPS/2022/001).
utb.wos.affiliation [Steinerova, Denisa; Kalendova, Andrea; Machotova, Jana] Univ Pardubice, Fac Chem Technol, Inst Chem & Technol Macromol Mat, Pardubice 53210, Czech Republic; [Knotek, Petr] Univ Pardubice, Fac Chem Technol, Dept Gen & Inorgan Chem, Pardubice 53210, Czech Republic; [Humpolicek, Petr; Vajdak, Jan] Tomas Bata Univ Zlin, Ctr Polymer Syst, Zlin 76001, Czech Republic; [Slang, Stanislav] Univ Pardubice, Fac Chem Technol, Ctr Mat & Nanotechnol, Pardubice 53210, Czech Republic; [Krejcova, Anna] Univ Pardubice, Fac Chem Technol, Inst Environm & Chem Engn, Pardubice 53210, Czech Republic; [Benes, Ludvik] Univ Pardubice, Fac Chem Technol, Joint Lab Solid State Chem, Pardubice 53210, Czech Republic; [Wolff-Fabris, Felipe] European Ctr Dispers Technol, D-95100 Selb, Germany
utb.scopus.affiliation Institute of Chemistry and Technology of Macromolecular Materials, Faculty of Chemical Technology, University of Pardubice, Pardubice, 532 10, Czech Republic; Department of General and Inorganic Chemistry, Faculty of Chemical Technology, University of Pardubice, Pardubice, 532 10, Czech Republic; Centre of Polymer Systems, Tomas Bata University in Zlín, Zlín, 760 01, Czech Republic; Center of Materials and Nanotechnologies, Faculty of Chemical Technology, University of Pardubice, Pardubice, 532 10, Czech Republic; Institute of Environmental and Chemical Engineering, Faculty of Chemical Technology, University of Pardubice, Pardubice, 532 10, Czech Republic; Joint Laboratory of Solid State Chemistry, Faculty of Chemical Technology, University of Pardubice, Pardubice, 532 10, Czech Republic; European Center for Dispersion Technologies, Selb, 95100, Germany
utb.fulltext.projects MSM LM2018103
utb.fulltext.projects RP/CPS/2022/001
utb.fulltext.faculty University Institute
utb.fulltext.faculty University Institute
utb.fulltext.ou Centre of Polymer Systems
utb.fulltext.ou Centre of Polymer Systems
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