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Effect of nano-sized poly(butyl acrylate) layer grafted from graphene oxide sheets on the compatibility and beta-phase development of poly(vinylidene fluoride) and their vibration sensing performance

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dc.title Effect of nano-sized poly(butyl acrylate) layer grafted from graphene oxide sheets on the compatibility and beta-phase development of poly(vinylidene fluoride) and their vibration sensing performance en
dc.contributor.author Mrlík, Miroslav
dc.contributor.author Ilčíková, Markéta
dc.contributor.author Osička, Josef
dc.contributor.author Kutálková, Erika
dc.relation.ispartof International Journal of Molecular Sciences
dc.identifier.issn 1661-6596 Scopus Sources, Sherpa/RoMEO, JCR
dc.identifier.issn 1422-0067 Scopus Sources, Sherpa/RoMEO, JCR
dc.date.issued 2022-05-21
utb.relation.volume 23
utb.relation.issue 10
dc.citation.spage 5777
dc.type article
dc.language.iso en
dc.publisher MDPI
dc.identifier.doi 10.3390/ijms23105777
dc.relation.uri https://www.mdpi.com/1422-0067/23/10/5777
dc.subject SI-ATRP en
dc.subject graphene oxide en
dc.subject poly(vinylidene fluoride) en
dc.subject dielectric properties en
dc.subject compatibility en
dc.subject vibration sensing en
dc.subject d(33) en
dc.description.abstract In this work, graphene oxide (GO) particles were modified with a nano-sized poly(butyl acrylate) (PBA) layer to improve the hydrophobicity of the GO and improve compatibility with PVDF. The improved hydrophobicity was elucidated using contact angle investigations, and exhibit nearly 0 degrees for neat GO and 102 degrees for GO-PBA. Then, the neat GO and GO-PBA particles were mixed with PVDF using a twin screw laboratory extruder. It was clearly shown that nano-sized PBA layer acts as plasticizer and shifts glass transition temperature from -38.7 degrees C for neat PVDF to 45.2 degrees C for PVDF/GO-PBA. Finally, the sensitivity to the vibrations of various frequencies was performed and the piezoelectric constant in the thickness mode, d(33), was calculated and its electrical load independency were confirmed. Received values of the d(33) were for neat PVDF 14.7 pC/N, for PVDF/GO 20.6 pC/N and for PVDF/GO-PBA 26.2 pC/N showing significant improvement of the vibration sensing and thus providing very promising systems for structural health monitoring and data harvesting. en
utb.faculty University Institute
utb.faculty Faculty of Technology
dc.identifier.uri http://hdl.handle.net/10563/1010995
utb.identifier.obdid 43884106
utb.identifier.scopus 2-s2.0-85130308653
utb.identifier.wok 000801952700001
utb.identifier.pubmed 35628584
utb.source J-wok
dc.date.accessioned 2022-06-10T07:48:32Z
dc.date.available 2022-06-10T07:48:32Z
dc.description.sponsorship Czech Science Foundation [19-17457S]; Ministry of Education, Youth and Sports of the Czech Republic-DKRVO [RP/CPS/2022/003]
dc.description.sponsorship RP/CPS/2022/003; Ministerstvo Školství, Mládeže a Tělovýchovy, MŠMT; Grantová Agentura České Republiky, GA ČR: 19-17457S
dc.rights Attribution 4.0 International
dc.rights.uri https://creativecommons.org/licenses/by/4.0/
dc.rights.access openAccess
utb.ou Centre of Polymer Systems
utb.ou Department of Physics and Materials Engineering
utb.contributor.internalauthor Mrlík, Miroslav
utb.contributor.internalauthor Ilčíková, Markéta
utb.contributor.internalauthor Osička, Josef
utb.contributor.internalauthor Kutálková, Erika
utb.fulltext.affiliation Miroslav Mrlik 1,* https://orcid.org/0000-0001-6203-6795 , Markéta Ilčíková 1,2,3,*, Josef Osička 1 https://orcid.org/0000-0002-4909-9350 and Erika Kutálková 1 1 Centre of Polymer Systems, Tomas Bata University in Zlin, 760 01 Zlin, Czech Republic; osicka@utb.cz (J.O.); ekutalkova@utb.cz (E.K.) 2 Polymer Institute, Slovak Academy of Sciences, Dubravska cesta 9, 845 45 Bratislava, Slovakia 3 Department of Physics and Materials Engineering, Faculty of Technology, Tomas Bata University in Zlin, 760 01 Zlin, Czech Republic * Correspondence: mrlik@utb.cz (M.M.); ilcikova@utb.cz (M.I.)
utb.fulltext.dates Received: 20 April 2022 Accepted: 17 May 2022 Published: 21 May 2022
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utb.fulltext.sponsorship Authors acknowledge the Czech Science Foundation grant No. 19-17457S for the financial support. The authors also gratefully acknowledge the Ministry of Education, Youth and Sports of the Czech Republic-DKRVO (RP/CPS/2022/003).
utb.wos.affiliation [Mrlik, Miroslav; Ilcikova, Marketa; Osicka, Josef; Kutalkova, Erika] Tomas Bata Univ Zlin, Ctr Polymer Syst, Zlin 76001, Czech Republic; [Ilcikova, Marketa] Slovak Acad Sci, Polymer Inst, Dubrayska Cesta 9, Bratislava 84545, Slovakia; [Ilcikova, Marketa] Tomas Bata Univ Zlin, Fac Technol, Dept Phys & Mat Engn, Zlin 76001, Czech Republic
utb.scopus.affiliation Centre of Polymer Systems, Tomas Bata University in Zlin, Zlin, 760 01, Czech Republic; Polymer Institute, Slovak Academy of Sciences, Dubravska cesta 9, Bratislava, 845 45, Slovakia; Department of Physics and Materials Engineering, Faculty of Technology, Tomas Bata University in Zlin, Zlin, 760 01, Czech Republic
utb.fulltext.projects 19-17457S
utb.fulltext.projects RP/CPS/2022/003
utb.fulltext.faculty University Institute
utb.fulltext.faculty Faculty of Technology
utb.fulltext.ou Centre of Polymer Systems
utb.fulltext.ou Department of Physics and Materials Engineering
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